TY - JOUR
T1 - Measurement of ambient PAHs in Kumamoto
T2 - Differentiating local and transboundary air pollution
AU - Sugiyama, Taichi
AU - Shimada, Kojiro
AU - Miura, Kaori
AU - Lin, Neng Huei
AU - Kim, Yong Pyo
AU - Chan, Chak K.
AU - Takami, Akinori
AU - Hatakeyama, Shiro
N1 - Publisher Copyright:
© Taiwan Association for Aerosol Research.
PY - 2017/12
Y1 - 2017/12
N2 - We developed an index to investigate the effect of transboundary air pollution (TAP) on the air quality of Kumamoto City, Japan. We estimated the effect of TAP by using the index and positive matrix factorization (PMF). Polycyclic aromatic hydrocarbons (PAHs) and trace metals were analyzed from the daily samples of the Total Suspended Particles (TSPs) collected seasonally from Oct. 2014 to Aug. 2015. These chemical components exhibited high concentrations in spring and winter, which is consistent with the data in the literature. Pb was identified as the TAP tracer owing to its high concentrations in winter and spring. Indeno(1, 2, 3-cd)pyrene (IcdP) was used as the local emission tracer in Kumamoto on the basis of previous studies. We applied the IcdP/Pb ratio as the index. The index enables the detection of TAP in daily data sets. PMF identified six factors: soil and road dust, biomass and waste burning, heavy oil combustion, fishing boats, vehicle emission, and coal combustion. The average contribution of TAP on the days when transboundary pollution was high was evaluated as being 46%.
AB - We developed an index to investigate the effect of transboundary air pollution (TAP) on the air quality of Kumamoto City, Japan. We estimated the effect of TAP by using the index and positive matrix factorization (PMF). Polycyclic aromatic hydrocarbons (PAHs) and trace metals were analyzed from the daily samples of the Total Suspended Particles (TSPs) collected seasonally from Oct. 2014 to Aug. 2015. These chemical components exhibited high concentrations in spring and winter, which is consistent with the data in the literature. Pb was identified as the TAP tracer owing to its high concentrations in winter and spring. Indeno(1, 2, 3-cd)pyrene (IcdP) was used as the local emission tracer in Kumamoto on the basis of previous studies. We applied the IcdP/Pb ratio as the index. The index enables the detection of TAP in daily data sets. PMF identified six factors: soil and road dust, biomass and waste burning, heavy oil combustion, fishing boats, vehicle emission, and coal combustion. The average contribution of TAP on the days when transboundary pollution was high was evaluated as being 46%.
KW - Contribution of local air pollution
KW - Contribution of transboundary air pollution
KW - Indeno(1, 2, 3-cd)pyrene
KW - Lead
KW - PMF analysis
UR - http://www.scopus.com/inward/record.url?scp=85037534261&partnerID=8YFLogxK
U2 - 10.4209/aaqr.2016.12.0585
DO - 10.4209/aaqr.2016.12.0585
M3 - Article
AN - SCOPUS:85037534261
SN - 1680-8584
VL - 17
SP - 3106
EP - 3118
JO - Aerosol and Air Quality Research
JF - Aerosol and Air Quality Research
IS - 12
ER -
