TY - JOUR
T1 - Fine particle measurements at two background sites in Korea between 1996 and 1997
AU - Lee, Jong Hoon
AU - Kim, Yong Pyo
AU - Moon, Kil Choo
AU - Kim, Hui Kang
AU - Lee, Chong Bum
N1 - Funding Information:
This work was supported by National Institute of Environmental Research, Korea. The authors thank Dr. Fung at AtmAA, USA for organic and elemental carbon analyses.
PY - 2001
Y1 - 2001
N2 - Five intensive field measurements were carried out at two background sites in Korea; Kosan and Kangwha during spring, fall, and winters of 1996 and 1997 to investigate the characteristics of long-range transport of air pollutants in northeastern Asia. Fine particles (PM2.5) were collected by low-volume samplers and the concentrations of major ions, organic and elemental carbons, and nitric acid were quantified. The concentrations of anthropogenic species in PM2.5 measured at both sites were generally higher than those at other background areas, Nagano, Japan and San Nicolas Is., USA due to continental outflow of air pollutants, but lower than those at an urban background site, Qingdao, China. The major components of PM2.5 were sulfate, organic carbon (OC), and ammonium for Kosan and sulfate, OC, ammonium, and nitrate for Kangwha. The major fractions of sulfate at both sites are non-sea-salts (nss) sulfate. Based on the relationship among major anthropogenic species, analysis of the nss sulfate to total nitrate molar ratios, and backward air parcel trajectories, it was found that fine particles measured at both sites during the measurement periods are mainly coming from China. At Kosan, the concentrations of anthropogenic species were higher when air parcels were coming from southern China than when air parcels were from northern China. At Kangwha, however, the differences of the concentrations were not statistically significant since most air parcels were from northern China and local effects are prominent. Copyright (C) 2001 Elsevier Science Ltd.
AB - Five intensive field measurements were carried out at two background sites in Korea; Kosan and Kangwha during spring, fall, and winters of 1996 and 1997 to investigate the characteristics of long-range transport of air pollutants in northeastern Asia. Fine particles (PM2.5) were collected by low-volume samplers and the concentrations of major ions, organic and elemental carbons, and nitric acid were quantified. The concentrations of anthropogenic species in PM2.5 measured at both sites were generally higher than those at other background areas, Nagano, Japan and San Nicolas Is., USA due to continental outflow of air pollutants, but lower than those at an urban background site, Qingdao, China. The major components of PM2.5 were sulfate, organic carbon (OC), and ammonium for Kosan and sulfate, OC, ammonium, and nitrate for Kangwha. The major fractions of sulfate at both sites are non-sea-salts (nss) sulfate. Based on the relationship among major anthropogenic species, analysis of the nss sulfate to total nitrate molar ratios, and backward air parcel trajectories, it was found that fine particles measured at both sites during the measurement periods are mainly coming from China. At Kosan, the concentrations of anthropogenic species were higher when air parcels were coming from southern China than when air parcels were from northern China. At Kangwha, however, the differences of the concentrations were not statistically significant since most air parcels were from northern China and local effects are prominent. Copyright (C) 2001 Elsevier Science Ltd.
KW - Ammonium to nss sulfate ratio
KW - Long-range transport
KW - Northeastern Asia
KW - Nss sulfate to nitrate ratio
KW - PM
UR - http://www.scopus.com/inward/record.url?scp=0035251668&partnerID=8YFLogxK
U2 - 10.1016/S1352-2310(00)00378-2
DO - 10.1016/S1352-2310(00)00378-2
M3 - Article
AN - SCOPUS:0035251668
SN - 1352-2310
VL - 35
SP - 635
EP - 643
JO - Atmospheric Environment
JF - Atmospheric Environment
IS - 4
ER -