Experimental and theoretical study of third-order harmonic generation in carbon nanotubes

Catrinel Stanciu, R. Ehlich, V. Petrov, O. Steinkellner, J. Herrmann, I. V. Hertel, G. Ya Slepyan, A. A. Khrutchinski, S. A. Maksimenko, F. Rotermund, E. E.B. Campbell, F. Rohmund

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Abstract

Third-order harmonic generation in carbon nanotubes was investigated using ultrashort pulses generated by a Cr:Forsterite laser, at a wavelength of 1250 nm. An unusual nonperturbative behavior of the third-harmonic yield was found for relatively low input laser fields, of ∼1010 W/cm2. Results showed that in a full quantum-mechanical theory for harmonics generation from a single-walled carbon nanotubes, there was strong nonlinearity of the laser interaction with carbon nanotubes.

Original languageEnglish
Pages (from-to)4064-4066
Number of pages3
JournalApplied Physics Letters
Volume81
Issue number21
DOIs
StatePublished - 18 Nov 2002

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