Electric-Field-Driven Spin Resonance by On-Surface Exchange Coupling to a Single-Atom Magnet

Soo hyon Phark, Hong Thi Bui, Alejandro Ferrón, Joaquin Fernández-Rossier, Jose Reina-Gálvez, Christoph Wolf, Yu Wang, Kai Yang, Andreas J. Heinrich, Christopher P. Lutz

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4 Scopus citations


Coherent control of individual atomic and molecular spins on surfaces has recently been demonstrated by using electron spin resonance (ESR) in a scanning tunneling microscope (STM). Here, a combined experimental and modeling study of the ESR of a single hydrogenated Ti atom that is exchange-coupled to a Fe adatom positioned 0.6–0.8 nm away by means of atom manipulation is presented. Continuous wave and pulsed ESR of the Ti spin show a Rabi rate with two contributions, one from the tip and the other from the Fe, whose spin interactions with Ti are modulated by the radio-frequency electric field. The Fe contribution is comparable to the tip, as revealed by its dominance when the tip is retracted, and tunable using a vector magnetic field. The new ESR scheme allows on-surface individual spins to be addressed and coherently controlled without the need for magnetic interaction with a tip. This study establishes a feasible implementation of spin-based multi-qubit systems on surfaces.

Original languageEnglish
Article number2302033
JournalAdvanced Science
Issue number27
StatePublished - 26 Sep 2023

Bibliographical note

Publisher Copyright:
© 2023 The Authors. Advanced Science published by Wiley-VCH GmbH.


  • Rabi rate
  • atom manipulation
  • electron spin resonance
  • scanning tunneling microscopy
  • single spin qubit
  • single-atom magnet


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