Effect of magnesium ion distinguishing between one-step hydrogen- and electron-transfer mechanisms for the reduction of stable neutral radicals by NADH analogues

Shunichi Fukuzumi, Yoshihiro Tokuda, Yutaka Chiba, Lucedio Greci, Patricia Carloni, Elisabetta Damiani

Research output: Contribution to journalArticlepeer-review

20 Scopus citations

Abstract

Hydrogen transfer from NADH analogues to indolinone and phenyliminoindolinone aminoxyl radicals proceeds via a one-step hydrogen-transfer process, in which no catalytic effect of Mg2+ has been observed, while the hydrogen transfer to 1,1-diphenyl-2-picrylhydrazyl radical proceeds via electron transfer from NADH analogues to the radical, which is catalyzed significantly by the presence of Mg2+ in MeCN.

Original languageEnglish
Pages (from-to)1575-1577
Number of pages3
JournalJournal of the Chemical Society, Chemical Communications
Issue number20
DOIs
StatePublished - 1993

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