Charge dynamics in a donor-acceptor covalent organic framework with periodically ordered bicontinuous heterojunctions

Shangbin Jin; Xuesong Ding; Xiao Feng; Mustafa Supur; Ko Furukawa; Seiya Takahashi; Matthew Addicoat; Mohamed E. El-Khouly; Toshikazu Nakamura; Stephan Irle; Shunichi Fukuzumi; Atsushi Nagai; Donglin Jiang

doi:10.1002/anie.201209513

Charge dynamics in a donor-acceptor covalent organic framework with periodically ordered bicontinuous heterojunctions

Shangbin Jin, Xuesong Ding, Xiao Feng, Mustafa Supur, Ko Furukawa, Seiya Takahashi, Matthew Addicoat, Mohamed E. El-Khouly, Toshikazu Nakamura, Stephan Irle, Shunichi Fukuzumi, Atsushi Nagai, Donglin Jiang

Department of Chemistry & Nanoscience

Research output: Contribution to journal › Article › peer-review

263 Scopus citations

Abstract

Light works: Mechanistic insights into the photochemical events and charge dynamics of a donor-acceptor covalent organic framework were given by time-resolved transient absorption spectroscopy and time-resolved electron spin resonance spectroscopy (see picture). The organic framework triggers ultrafast electron transfer and enables long-distance charge delocalization and exceptional long-term charge separation.

Original language	English
Pages (from-to)	2017-2021
Number of pages	5
Journal	Angewandte Chemie - International Edition
Volume	52
Issue number	7
DOIs	https://doi.org/10.1002/anie.201209513
State	Published - 11 Feb 2013

Keywords

acceptor
charge dynamics
donor
electron transfer
organic frameworks

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10.1002/anie.201209513

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Jin, S., Ding, X., Feng, X., Supur, M., Furukawa, K., Takahashi, S., Addicoat, M., El-Khouly, M. E., Nakamura, T., Irle, S., Fukuzumi, S., Nagai, A., & Jiang, D. (2013). Charge dynamics in a donor-acceptor covalent organic framework with periodically ordered bicontinuous heterojunctions. Angewandte Chemie - International Edition, 52(7), 2017-2021. https://doi.org/10.1002/anie.201209513

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abstract = "Light works: Mechanistic insights into the photochemical events and charge dynamics of a donor-acceptor covalent organic framework were given by time-resolved transient absorption spectroscopy and time-resolved electron spin resonance spectroscopy (see picture). The organic framework triggers ultrafast electron transfer and enables long-distance charge delocalization and exceptional long-term charge separation.",

keywords = "acceptor, charge dynamics, donor, electron transfer, organic frameworks",

author = "Shangbin Jin and Xuesong Ding and Xiao Feng and Mustafa Supur and Ko Furukawa and Seiya Takahashi and Matthew Addicoat and El-Khouly, {Mohamed E.} and Toshikazu Nakamura and Stephan Irle and Shunichi Fukuzumi and Atsushi Nagai and Donglin Jiang",

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doi = "10.1002/anie.201209513",

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Jin, S, Ding, X, Feng, X, Supur, M, Furukawa, K, Takahashi, S, Addicoat, M, El-Khouly, ME, Nakamura, T, Irle, S, Fukuzumi, S, Nagai, A & Jiang, D 2013, 'Charge dynamics in a donor-acceptor covalent organic framework with periodically ordered bicontinuous heterojunctions', Angewandte Chemie - International Edition, vol. 52, no. 7, pp. 2017-2021. https://doi.org/10.1002/anie.201209513

TY - JOUR

T1 - Charge dynamics in a donor-acceptor covalent organic framework with periodically ordered bicontinuous heterojunctions

AU - Jin, Shangbin

AU - Ding, Xuesong

AU - Feng, Xiao

AU - Supur, Mustafa

AU - Furukawa, Ko

AU - Takahashi, Seiya

AU - Addicoat, Matthew

AU - El-Khouly, Mohamed E.

AU - Nakamura, Toshikazu

AU - Irle, Stephan

AU - Fukuzumi, Shunichi

AU - Nagai, Atsushi

AU - Jiang, Donglin

PY - 2013/2/11

Y1 - 2013/2/11

N2 - Light works: Mechanistic insights into the photochemical events and charge dynamics of a donor-acceptor covalent organic framework were given by time-resolved transient absorption spectroscopy and time-resolved electron spin resonance spectroscopy (see picture). The organic framework triggers ultrafast electron transfer and enables long-distance charge delocalization and exceptional long-term charge separation.

AB - Light works: Mechanistic insights into the photochemical events and charge dynamics of a donor-acceptor covalent organic framework were given by time-resolved transient absorption spectroscopy and time-resolved electron spin resonance spectroscopy (see picture). The organic framework triggers ultrafast electron transfer and enables long-distance charge delocalization and exceptional long-term charge separation.

KW - acceptor

KW - charge dynamics

KW - donor

KW - electron transfer

KW - organic frameworks

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DO - 10.1002/anie.201209513

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VL - 52

SP - 2017

EP - 2021

JO - Angewandte Chemie - International Edition

JF - Angewandte Chemie - International Edition

IS - 7

ER -

Charge dynamics in a donor-acceptor covalent organic framework with periodically ordered bicontinuous heterojunctions

Abstract

Keywords

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